Project 01
High Performance CO2 Capture Module
2023 / Experimental Systems / Thesis
Minimizing the energy required for post-combustion CO₂ capture is critical to reducing the cost of industrial decarbonization. Conventional capture technologies, including absorption, membranes, and packed-bed adsorption, face challenges related to high energy demand, temperature requirements, scalability, and site dependence. Adsorption offers a lower-energy alternative, but conventional packed beds suffer from poor heat transfer and often rely on electricity-intensive vacuum regeneration. This study develops and demonstrates an adsorbent-coated microchannel heat exchanger designed for rapid, heat-driven CO₂ capture and regeneration. The system uses aluminum microchannel plates coated with Zeolite 13X and interlayered with uncoated microchannel plates carrying a heat-transfer fluid. A coating formulation using xanthan gum as a binder was developed to provide strong adhesion while preserving adsorbent porosity. The dehydrated coating contained 97.6–98% Zeolite 13X and 2–2.4% binder, with SEM imaging showing minimal impact on the characteristic zeolite pore structure. The final system contained seven coated plates with 21.84 g of Zeolite 13X, paired with 1 mm heat-transfer plates and custom headers and silicone gaskets for independent gas and liquid flow. CO₂ capture experiments were conducted using a 20% CO₂/80% N₂ gas mixture and a Raman laser gas analyzer. Regeneration was achieved by circulating 50–65°C water through the heat-transfer channels - temperatures equivalent to low grade waste heat from numerous industrial sectors. System performance was evaluated based on CO₂ adsorption capacity, adsorbent mass, bed volume, and thermal energy required for regeneration. The results demonstrate the potential of coated microchannel architectures to provide a compact, scalable, and low-temperature approach to adsorption-based CO₂ capture, resulting in 3 times faster desorption rates.
Key Contributions
- 01Designed full system
- 02Manufactured, and assembled full assembly
- 03Formulated coatings
- 04Validated System through experimentation
- 05Ran the test campaign and reported capture capacity
- Role
- Thesis
- Tools
- Fusion 360 / Python / LabVIEW / COMSOL / Water-jet / Laser Cutter / Standard machining
- System
- Thermal / Experimental
- Year
- 2023
- Thermal Systems
- Experimental
- Energy
- CO2 Capture
